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NPR's Invisibilia. My coworkers and I were obsessed with this one last summer, and it sparked some really interesting conversations.
Ologies is a series of conversations with scientists!!
That Classical Podcast is a bit of a music-nerd-specific thing but it's hilarious and interesting. Highly recommend if you're even mildly interested in classical music.
Also, in French: Transfert is a random storytelling podcast and it's made my bus commutes more bearable recently!